The Effect of CO2 Availability on the Growth, Iron Oxidation and CO2-Fixation Rates of Pure Cultures of Leptospirillum ferriphilum and Acidithiobacillus ferrooxidans

dc.contributor.authorBryan, C G
dc.contributor.authorDavis-Belmar, C S
dc.contributor.authorvan Wyk, N
dc.contributor.authorFraser, M K
dc.contributor.authorDew, D
dc.contributor.authorRautenbach, G F
dc.contributor.authorHarrison, S T L
dc.date.accessioned2016-08-18T11:39:09Z
dc.date.available2016-08-18T11:39:09Z
dc.date.issued2012
dc.date.updated2016-08-17T11:01:45Z
dc.description.abstractUnderstanding how bioleaching systems respond to the availability of CO2 is essential to developing operating conditions that select for optimum microbial performance. Therefore, the effect of inlet gas and associated dissolved CO2 concentration on the growth, iron oxidation and CO2-fixation rates of pure cultures of Acidithiobacillus ferrooxidans and Leptospirillum ferriphilum was investigated in a batch stirred tank system. The minimum inlet CO2 concentrations required to promote the growth of At. ferrooxidans and L. ferriphilum were 25 and 70 ppm, respectively, and corresponded to dissolved CO2 concentrations of 0.71 and 1.57 mM (at 308C and 378C, respectively). An actively growing culture of L. ferriphilum was able to maintain growth at inlet CO2 concentrations less than 30 ppm (0.31–0.45 mM in solution). The highest total new cell production and maximum specific growth rates from the stationary phase inocula were observed with CO2 inlet concentrations less than that of air. In contrast, the amount of CO2 fixed per new cell produced increased with increasing inlet CO2 concentrations above 100 ppm. Where inlet gas CO2 concentrations were increased above that of air the additional CO2 was consumed by the organisms but did not lead to increased cell production or significantly increase performance in terms of iron oxidation. It is proposed that At. ferrooxidans has two CO2 uptake mechanisms, a high affinity system operating at low available CO2 concentrations, which is subject to substrate inhibition and a low affinity system operating at higher available CO2 concentrations. L. ferriphilum has a single uptake system characterised by a moderate CO2 affinity. At. ferrooxidans performed better than L. ferriphilum at lower CO2 availabilities, and was less affected by CO2 starvation. Finally, the results demonstrate the limitations of using CO2 uptake or ferrous iron oxidation data as indirect measures of cell growth and performance across varying physiological conditions. Biotechnol. Bioeng. 2012;109: 1693–1703en_ZA
dc.identifierhttp://dx.doi.org/10.1002/bit.24453
dc.identifier.apacitationBryan, C. G., Davis-Belmar, C. S., van Wyk, N., Fraser, M. K., Dew, D., Rautenbach, G. F., & Harrison, S. T. L. (2012). The Effect of CO2 Availability on the Growth, Iron Oxidation and CO2-Fixation Rates of Pure Cultures of Leptospirillum ferriphilum and Acidithiobacillus ferrooxidans. <i>Biotechnology and Bioengineering</i>, http://hdl.handle.net/11427/21316en_ZA
dc.identifier.chicagocitationBryan, C G, C S Davis-Belmar, N van Wyk, M K Fraser, D Dew, G F Rautenbach, and S T L Harrison "The Effect of CO2 Availability on the Growth, Iron Oxidation and CO2-Fixation Rates of Pure Cultures of Leptospirillum ferriphilum and Acidithiobacillus ferrooxidans." <i>Biotechnology and Bioengineering</i> (2012) http://hdl.handle.net/11427/21316en_ZA
dc.identifier.citationBryan, C. G., Davis‐Belmar, C. S., van Wyk, N., Fraser, M. K., Dew, D., Rautenbach, G. F., & Harrison, S. T. L. (2012). The effect of CO2 availability on the growth, iron oxidation and CO2‐fixation rates of pure cultures of Leptospirillum ferriphilum and Acidithiobacillus ferrooxidans. Biotechnology and bioengineering, 109(7), 1693-1703.en_ZA
dc.identifier.issn0006-3592en_ZA
dc.identifier.ris TY - Journal Article AU - Bryan, C G AU - Davis-Belmar, C S AU - van Wyk, N AU - Fraser, M K AU - Dew, D AU - Rautenbach, G F AU - Harrison, S T L AB - Understanding how bioleaching systems respond to the availability of CO2 is essential to developing operating conditions that select for optimum microbial performance. Therefore, the effect of inlet gas and associated dissolved CO2 concentration on the growth, iron oxidation and CO2-fixation rates of pure cultures of Acidithiobacillus ferrooxidans and Leptospirillum ferriphilum was investigated in a batch stirred tank system. The minimum inlet CO2 concentrations required to promote the growth of At. ferrooxidans and L. ferriphilum were 25 and 70 ppm, respectively, and corresponded to dissolved CO2 concentrations of 0.71 and 1.57 mM (at 308C and 378C, respectively). An actively growing culture of L. ferriphilum was able to maintain growth at inlet CO2 concentrations less than 30 ppm (0.31–0.45 mM in solution). The highest total new cell production and maximum specific growth rates from the stationary phase inocula were observed with CO2 inlet concentrations less than that of air. In contrast, the amount of CO2 fixed per new cell produced increased with increasing inlet CO2 concentrations above 100 ppm. Where inlet gas CO2 concentrations were increased above that of air the additional CO2 was consumed by the organisms but did not lead to increased cell production or significantly increase performance in terms of iron oxidation. It is proposed that At. ferrooxidans has two CO2 uptake mechanisms, a high affinity system operating at low available CO2 concentrations, which is subject to substrate inhibition and a low affinity system operating at higher available CO2 concentrations. L. ferriphilum has a single uptake system characterised by a moderate CO2 affinity. At. ferrooxidans performed better than L. ferriphilum at lower CO2 availabilities, and was less affected by CO2 starvation. Finally, the results demonstrate the limitations of using CO2 uptake or ferrous iron oxidation data as indirect measures of cell growth and performance across varying physiological conditions. Biotechnol. Bioeng. 2012;109: 1693–1703 DA - 2012 DB - OpenUCT DP - University of Cape Town J1 - Biotechnology and Bioengineering LK - https://open.uct.ac.za PB - University of Cape Town PY - 2012 SM - 0006-3592 T1 - The Effect of CO2 Availability on the Growth, Iron Oxidation and CO2-Fixation Rates of Pure Cultures of Leptospirillum ferriphilum and Acidithiobacillus ferrooxidans TI - The Effect of CO2 Availability on the Growth, Iron Oxidation and CO2-Fixation Rates of Pure Cultures of Leptospirillum ferriphilum and Acidithiobacillus ferrooxidans UR - http://hdl.handle.net/11427/21316 ER - en_ZA
dc.identifier.urihttp://hdl.handle.net/11427/21316
dc.identifier.vancouvercitationBryan CG, Davis-Belmar CS, van Wyk N, Fraser MK, Dew D, Rautenbach GF, et al. The Effect of CO2 Availability on the Growth, Iron Oxidation and CO2-Fixation Rates of Pure Cultures of Leptospirillum ferriphilum and Acidithiobacillus ferrooxidans. Biotechnology and Bioengineering. 2012; http://hdl.handle.net/11427/21316.en_ZA
dc.languageengen_ZA
dc.publisherWileyen_ZA
dc.publisher.institutionUniversity of Cape Town
dc.sourceBiotechnology and Bioengineeringen_ZA
dc.source.urihttp://onlinelibrary.wiley.com/journal/10.1002/(ISSN)1097-0290
dc.subject.otherBioleaching
dc.subject.otherCO2-fixation
dc.subject.otherIron oxidation
dc.subject.otherGrowth rate
dc.subject.otherAcidithiobacillus ferrooxidans
dc.titleThe Effect of CO2 Availability on the Growth, Iron Oxidation and CO2-Fixation Rates of Pure Cultures of Leptospirillum ferriphilum and Acidithiobacillus ferrooxidansen_ZA
dc.typeJournal Articleen_ZA
uct.type.filetypeText
uct.type.filetypeImage
uct.type.publicationResearchen_ZA
uct.type.resourceArticleen_ZA
Files
Original bundle
Now showing 1 - 1 of 1
Loading...
Thumbnail Image
Name:
Bryan_Effect_CO2_2012.pdf
Size:
335.23 KB
Format:
Adobe Portable Document Format
Description:
License bundle
Now showing 1 - 1 of 1
Loading...
Thumbnail Image
Name:
license.txt
Size:
1.72 KB
Format:
Item-specific license agreed upon to submission
Description:
Collections